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Tsujimoto, Kazufumi; Oigawa, Hiroyuki; Shinohara, Nobuo
Proceedings of International Conference on Nuclear Data for Science and Technology (ND 2004), 4 Pages, 2004/09
Japan Atomic Energy Research Institute (JAERI) has been developing technologies for partitioning and transmutation of long-lived nuclides in high-level radioactive waste. In the dedicated transmutation systems, reliable neuclear data of minor actinide (MA) are indispensable to obtain a reliable design of a transmutation system. Present status of MA nuclear data is not so satisfactory. To obtain reliable nuclear data of MA, radiochemically analyzed data of the actinide samples irradiated at the Dounreay Prototype Fast Reactor (PFR) were used in this study. The samples were actinide oxides of 21 different isotopes from thorium to curium. The burnup calculations were performed and the calculated results were compared with the experimental data to validate the neutron cross section data of MA in an evaluated nuclear data file JENDL-3.3, ENDF/B-VI, and JEFF-3.0. The results for uraniumu and plutoniumu samples show good agreements with experimental data. On the other hand, in the results for americium and curiumu, relatively large disagreement with experimental data are showed.
Tsujimoto, Kazufumi; Kono, Nobuaki; Shinohara, Nobuo; Sakurai, Takeshi; Nakahara, Yoshinori; Mukaiyama, Takehiko; Raman, S.*
Nuclear Science and Engineering, 144(2), p.129 - 141, 2003/06
To evaluate neutron cross-section data of minor actinides, separated actinide samples and dosimetry samples were irradiated at the Dounreay Prototype Fast Reactor for 492 effective full power days. Based on the burnup calculations of major actinide and dosimetry samples, the neutron flux distribution and the flux level were adjusted at the locations where minor actinide samples were irradiated. The burnup calculations were carried out for minor actinides using the determined flux distribution and flux level. This paper discusses the burnup calculations and the validation of minor actinide cross-section data in evaluated nuclear data libraries. We find that we can obtain reliable FIMA (fission per initial metallic atom) values by using the 
Nd method except that the uncertainties in the FIMA values are large for 
U, 
Pu, Am isotopes, and Cm isotopes because the Nd yields are known poorly for these isotopes and are probably overestimated. For these isotopes, measurements to improve the fission-yield data are needed. We also find that, in general, the JENDL-3.2 nuclear data for the minor actinides are adequate for the conceptual design study of transmutation systems. But, there are some nuclides (especially Pu and 
Pu) for which new measurements are needed particulary if the minor actinides constitute a major part of the nuclear fuel.
